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Because ozone provides a shield against harmful ultraviolet radiation, determines the temperature profile in the stratosphere, plays important roles in tropospheric chemistry and climate, and is a health risk near the surface, changes in natural ozone layers at different altitudes and their global impact are being intensively researched. Global ozone coverage is currently provided by passive optical and microwave satellite sensors that cannot deliver high spatial resolution measurements and have particular limitations in the troposphere. Vertical profiling DIfferential Absorption Lidars (DIAL) have shown excellent range-resolved capabilities, but these systems have been large, inefficient, and have required continuous technical attention for long term operations. Recently, successful, autonomous DIAL measurements have been performed from a high-altitude aircraft (LASE - Lidar Atmospheric Sensing Experiment), and a space-qualified aerosol lidar system (LITE - Laser In-space Technology Experiment) has performed well on Shuttle. Based on the above successes, NASA and the Canadian Space Agency are jointly studying the feasibility of developing ORACLE (Ozone Research with Advanced Cooperative Lidar Experiments), an autonomously operated, compact DIAL instrument to be placed in orbit using a Pegasus class launch vehicle.

Atmospheric water vapor plays an important role in atmospheric chemistry and meteorology, with implications for climate change and severe weather. The Raman lidar technique is useful for observing water-vapor with high spatiotemporal resolutions. However, the calibration factor must be determined before observations. Because the calibration factor is generally evaluated by comparing Raman-signal results with those of independent measurement techniques (e.g., radiosonde), it is difficult to apply this technique to lidar sites where radiosonde observation cannot be carried out. In this study, we propose a new calibration technique for water-vapor Raman lidar using global navigation satellite system (GNSS)-derived precipitable water vapor (PWV) and Japan Meteorological Agency meso-scale model (MSM). The analysis was accomplished by fitting the GNSS-PWV to integrated water-vapor profiles combined with the MSM and the results of the lidar observations. The maximum height of the lidar signal applicable to this method was determined within 2.0 km by considering the signal noise mainly caused by low clouds. The MSM data was employed at higher regions that cannot apply the lidar data. This method can be applied to lidar signals lower than a limited height range due to weather conditions and lidar specifications. For example, Raman lidar using a laser operating in the ultraviolet C (UV-C) region has the advantage of daytime observation since there is no solar background radiation in the system. The observation range is, however, limited at altitudes lower than 1-3 km because of strong ozone absorption at the UV-C region. The new calibration technique will allow the utilization of various types of Raman lidar systems and provide many opportunities for calibration. We demonstrated the potential of this method by using the UV-C Raman lidar and GNSS observation data at the Shigaraki MU radar observatory (3451'N, 13606'E; 385m a.s.l.) of the Research Institute for Sustainable

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